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To facilitate an efficient electron transfer between PSP2 and catalysts and improve catalytic efficiency, N -(2,6,2-terpyridine-4-yl)iodoacetamide was attached covalently to the optimized mutant PSP2–95C93Y97Y with subsequent formation of a nickel (Ni II )–terpyridine complex (Figure 9c), resulting in a photocatalytic CO 2 -reducing enzyme termed as PSP2T2 with an impressive CO 2 /CO conversion quantum efficiency of 2.6%
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